金指 正言MASAKOTO KANEZASHI

Last Updated :2024/07/22

所属・職名
大学院先進理工系科学研究科 教授
ホームページ
メールアドレス
kanezashihiroshima-u.ac.jp
その他連絡先
東広島市鏡山一丁目4番1号 工学部A4棟213号室
TEL:082-424-2035 FAX:082-424-5494
自己紹介
近年,環境問題や省エネプロセスを実現するために,水素,二酸化炭素などの気体分離,エタノール水溶液からの脱水あるいは脱アルコールなどの液体混合物の分離,濾過分離など,膜分離プロセスが注目されています。私は,多孔性材料をベースにガス分離から液体分離まで分離対象に応じた膜開発と分離特性の評価について研究しています。特にアモルファスシリカを用いたサブナノレベルでの細孔径制御,吸着性制御などマイクロポーラス構造の制御技術を中心に研究を行なっています。

基本情報

主な職歴

  • 2005年10月01日, 2007年09月30日, アリゾナ州立大学, 工学部化学工学科, 博士研究員
  • 2007年10月01日, 2010年03月31日, 広島大学, 大学院工学研究科物質化学システム専攻, 助教
  • 2010年04月01日, 2017年02月28日, 広島大学, 大学院工学研究院物質化学工学部門, 助教
  • 2017年03月01日, 2020年03月31日, 広島大学, 大学院工学研究科化学工学専攻, 准教授
  • 2020年04月01日, 2022年09月30日, 広島大学, 大学院先進理工系科学研究科, 准教授
  • 2022年10月01日, 広島大学, 大学院先進理工系科学研究科, 教授

学位

  • 博士(工学) (広島大学)
  • 修士(工学) (広島大学)

教育担当

  • 【学士課程】 工学部 : 第三類(応用化学・生物工学・化学工学系) : 化学工学プログラム
  • 【博士課程前期】 先進理工系科学研究科 : 先進理工系科学専攻 : 化学工学プログラム
  • 【博士課程後期】 先進理工系科学研究科 : 先進理工系科学専攻 : 化学工学プログラム

研究分野

  • 工学 / プロセス・化学工学 / 化工物性・移動操作・単位操作

研究キーワード

  • ゾル-ゲル法
  • 膜分離工学
  • ガス分離
  • 細孔径制御
  • マイクロポーラス構造制御

所属学会

教育活動

授業担当

  1. 2024年, 教養教育, 1ターム, カーボンニュートラル推進科学
  2. 2024年, 学部専門, 2ターム, 物理化学I
  3. 2024年, 学部専門, セメスター(後期), 基礎化学実験
  4. 2024年, 学部専門, 2ターム, 基礎工業概論
  5. 2024年, 学部専門, セメスター(前期), 物質移動論
  6. 2024年, 学部専門, セメスター(前期), 化学工程設計
  7. 2024年, 学部専門, 通年, 卒業論文
  8. 2024年, 修士課程・博士課程前期, セメスター(前期), 化学工学特別演習A
  9. 2024年, 修士課程・博士課程前期, 3ターム, 化学工学特別演習B
  10. 2024年, 修士課程・博士課程前期, 4ターム, 化学工学特別演習B
  11. 2024年, 修士課程・博士課程前期, 年度, 化学工学特別研究
  12. 2024年, 修士課程・博士課程前期, 4ターム, 界面制御工学特論
  13. 2024年, 修士課程・博士課程前期, 3ターム, Advanced Surface Control Engineering
  14. 2024年, 博士課程・博士課程後期, 年度, 化学工学特別研究

教育に関する受賞

  • 2013年12月12日, 平成25年度広島大学大学院工学研究科・工学部教育顕彰, 広島大学, 第三類基礎化学実験(物理化学実験)における教育と実験環境の改善
  • 2017年11月16日, 平成29年度広島大学大学院工学研究科・工学部教育顕彰, 広島大学, 化学工学プログラミングにおけるテキスト作成とアクティブラーニングの実践

研究活動

学術論文(★は代表的な論文)

  1. Preparation of Polysilsesquioxane-Based CO2 Separation Membranes with Thermally Degradable Succinic Anhydride and Urea Units, SEPARATIONS, 11巻, 4号, 202404
  2. Network engineering of organosilica membranes for efficient pervaporation dehydration, SEPARATION AND PURIFICATION TECHNOLOGY, 344巻, 20240920
  3. Fabrication of 3-(trihydroxysilyl)-1-propanesulfonic acid membranes with superior affinity and selectivity for NH3 permeation over H2 and N2 at 50-300 °C, JOURNAL OF MEMBRANE SCIENCE, 702巻, 202405
  4. ★, Rigid-flexible coupled organosilica membranes toward high-efficiency molecules separation, JOURNAL OF MEMBRANE SCIENCE, 701巻, 202405
  5. Development of sulfonated (3-Mercaptopropyl)trimethoxysilane membranes with thermal stability and excellent NH3 perm-selectivity at 300 °C, JOURNAL OF MEMBRANE SCIENCE, 696巻, 202403
  6. Physicochemical Treatments of Graphene Oxide to Improve Water Vapor/Gas Separation Performance of Supported Laminar Membranes: Sonication and H2O2 Oxidation, ACS APPLIED MATERIALS & INTERFACES, 16巻, 6号, pp. 8086-8097, 20240201
  7. Permeation properties and hydrothermal stability of allylhydridopolycarbosilane (AHPCS)-derived silicon carbide (SiC) membranes, MATERIALS ADVANCES, 5巻, 6号, pp. 2420-2429, 20240318
  8. ★, Gas-Permeable Carbon Molecular Sieve Membranes Fabricated from a Norbornene-Functionalized Polyimide-Polyhedral Oligomeric Silsesquioxane Composite, INDUSTRIAL & ENGINEERING CHEMISTRY RESEARCH, 63巻, 3号, pp. 1554-1565, 20240110
  9. Bis(triethoxysilyl)ethane (BTESE)-Organosilica Membranes for H2O/DMF Separation in Reverse Osmosis (RO): Evaluation and Correlation of Subnanopores via Nanopermporometry (NPP), Modified Gas Translation (mGT) and RO Performance, MEMBRANES, 14巻, 1号, 202401
  10. 無機多孔膜を用いた超高圧RO/NFによる有機水溶液の高濃度濃縮, 膜(MEMBRANE), 49巻, pp. 7-12, 20240101
  11. Enhancement of water permeability in SiO2-ZrO2 nanofiltration membranes via adding organic solutes into the SiO2-ZrO2 sols, SEPARATION AND PURIFICATION TECHNOLOGY, 333巻, 20240401
  12. ★, Gas permeation properties of bridged-type organosilica membranes at extremely low temperatures and the application to oxygen separation, JOURNAL OF MEMBRANE SCIENCE, 691巻, 20240205
  13. Steam recovery from flue gas by organosilica membranes for simultaneous harvesting of water and energy, NATURE COMMUNICATIONS, 14巻, 1号, 20231123
  14. A highly water-selective carboxymethylated cellulose nanofiber (CNF-CMC) membrane for the separation of binary (water/N2) and ternary (water/alcohols/N2) systems in vapor-permeation, JOURNAL OF MEMBRANE SCIENCE, 691巻, 20240205
  15. Sub-nanometer scale tailoring of the microstructures of composite organosilica membranes for efficient pervaporation of toluene/ n-heptane mixtures, JOURNAL OF MEMBRANE SCIENCE, 672巻, 20230415
  16. Optimization of Ni-amine coordination for improving NH3 permeation through nickel-doped bis[3-(trimethoxysilyl)propyl] amine membranes, SEPARATION AND PURIFICATION TECHNOLOGY, 326巻, 20231201
  17. An ultrahigh permeance and CO2 selective membrane of organosilica-based coordination polymer tailored via nickel crosslinking, JOURNAL OF MEMBRANE SCIENCE, 679巻, 20230805
  18. Enhanced NH3 permeation of bis[3-(trimethoxysilyl)propyl] amine membranes via coordination with metals, JOURNAL OF MEMBRANE SCIENCE, 678巻, 20230715
  19. Steam permeation properties of perfluorosulfonic acid/ceramic composite membranes at a high temperature under various humidity conditions, SEPARATION AND PURIFICATION TECHNOLOGY, 320巻, 20230901
  20. ★, Catalytic effect of trifluoroacetic acid on the CO2 transport properties of organic-inorganic hybrid silica membranes, JOURNAL OF MEMBRANE SCIENCE LETTERS, 3巻, 1号, 202305
  21. Atmospheric-pressure plasma modification to control porous structure and affinity of organosilica membranes for pervaporation dehydration: Effect of plasma modification time, SEPARATION AND PURIFICATION TECHNOLOGY, 320巻, 20230901
  22. ★, A Brief Overview of the Microstructural Engineering of Inorganic-Organic Composite Membranes Derived from Organic Chelating Ligands, MEMBRANES, 13巻, 4号, 202304
  23. Permeation Properties of Water Vapor through Graphene Oxide/Polymer Substrate Composite Membranes, MEMBRANES, 13巻, 5号, 20230521
  24. ★, ゾル-ゲル法によりCO2親和性を制御したシリカ系多孔膜, MATERIAL STAGE, 23巻, pp. 27-33, 20230610
  25. Preparation of thermally stable 3-glycidyloxypropyl-POSS-derived polysilsesquioxane RO membranes for water desalination, JOURNAL OF MEMBRANE SCIENCE, 668巻, 20230215
  26. Preparation of urea- and isocyanurate-containing polysilsesquioxane membranes for CO2 separation, JOURNAL OF SOL-GEL SCIENCE AND TECHNOLOGY, 106巻, 1号, pp. 149-157, 202304
  27. ★, Hydrothermal Stability of Hydrogen-Selective Carbon-Ceramic Membranes Derived from Polybenzoxazine-Modified Silica-Zirconia, MEMBRANES, 13巻, 1号, 202301
  28. ★, The Effect of C/Si Ratio and Fluorine Doping on the Gas Permeation Properties of Pendant-Type and Bridged-Type Organosilica Membranes, MEMBRANES, 12巻, 10号, 202210
  29. Water permeation in gas and liquid phases through organosilica membranes: A unified theory of reverse osmosis, pervaporation, and vapor permeation, CHEMICAL ENGINEERING SCIENCE, 263巻, 20221214
  30. ★, Microporous structure control of SiO2-ZrO2 composite membranes via Yttrium doping and an evaluation of thermal stability, JOURNAL OF SOL-GEL SCIENCE AND TECHNOLOGY, 104巻, 3号, pp. 566-579, 202212
  31. Ammonia permeation of fluorinated sulfonic acid polymer/ceramic composite membranes, JOURNAL OF MEMBRANE SCIENCE, 658巻, 20220915
  32. Metal-Induced Aminosilica Rigidity Improves Highly Permeable Microporous Membranes via Different Types of Pendant Precursors, ACS APPLIED MATERIALS & INTERFACES, 14巻, 37号, pp. 42692-42704, 20220921
  33. Low-temperature cross-linking fabrication of sub-nanoporous SiC-based membranes for application to the pervaporation removal of methanol, JOURNAL OF MEMBRANE SCIENCE, 662巻, 20221015
  34. ★, Tailoring the structure of a sub-nano silica network via fluorine doping to enhance CO2 separation and evaluating CO2 separation performance under dry or wet conditions, JOURNAL OF MEMBRANE SCIENCE, 658巻, 20220915
  35. Transesterification membrane reactor with organosilica membrane in batch and continuous flow modes, CHEMICAL ENGINEERING JOURNAL, 450巻, 20221215
  36. Hydrophilic behavior of methyl-terminated organosilica thin films modified by atmospheric-pressure water vapor plasma, MATERIALS LETTERS, 325巻, 20221015
  37. ★, Design of carbon-ceramic composite membranes with tunable molecular cut-offs from a carboxylic benzoxazine ligand chelated to silica-zirconia, MOLECULAR SYSTEMS DESIGN & ENGINEERING, 7巻, 9号, 20220830
  38. Structural transformation of the nickel coordination-induced subnanoporosity of aminosilica membranes for methanol-selective, high-flux pervaporation, JOURNAL OF MEMBRANE SCIENCE, 656巻, 20220815
  39. Development of robust and high-performance polysilsesquioxane reverse osmosis membranes modified by SiO2 nanoparticles for water desalination, SEPARATION AND PURIFICATION TECHNOLOGY, 296巻, 20220901
  40. Nanogradient Hydrophilic/Hydrophobic Organosilica Membranes Developed by Atmospheric-Pressure Plasma to Enhance Pervaporation Performance, ACS NANO, 16巻, 7号, pp. 10302-10313, 20220726
  41. Open-air plasma deposition of polymer-supported silica-based membranes for, SEPARATION AND PURIFICATION TECHNOLOGY, 291巻, 20220615
  42. Preparation of amine- and ammonium-containing polysilsesquioxane membranes for CO2 separation, POLYMER JOURNAL, 54巻, 7号, pp. 875-882, 202207
  43. Development of Highly Water-Permeable Robust PSQ-Based RO Membranes by Introducing Hydroxyethylurea-Based Hydrophilic Water Channels, ACS APPLIED MATERIALS & INTERFACES, 14巻, 18号, pp. 21426-21435, 20220511
  44. Reverse osmosis and pervaporation of organic liquids using organosilica membranes: Performance analysis and predictions, AICHE JOURNAL, 68巻, 4号, 202204
  45. ★, Effect of fluorine doping on the network pore structure of non-porous organosilica bis(triethoxysilyl)propane (BTESP) membranes for use in molecular separation, JOURNAL OF MEMBRANE SCIENCE, 644巻, 20220215
  46. Network tailoring of organosilica membranes via aluminum doping to improve the humid-gas separation performance, RSC ADVANCES, 12巻, 10号, pp. 5834-5846, 20220216
  47. Development of PSQ-RO membranes with high water permeability by copolymerization of bis[3-(triethoxysilyl)propyl]amine and triethoxy (3-glycidyloxypropyl)silane, JOURNAL OF MEMBRANE SCIENCE, 644巻, 20220215
  48. ★, Boosting the CO2 capture efficiency through aromatic bridged organosilica membranes, JOURNAL OF MEMBRANE SCIENCE, 643巻, 20220301
  49. ★, Enhancement of the H-2-permselectivity of a silica-zirconia composite membrane enabled by ligand-ceramic to carbon-ceramic transformation, JOURNAL OF MEMBRANE SCIENCE, 642巻, 20220215
  50. Structural two-phase evolution of aminosilica-based silver-coordinated membranes for increased hydrogen separation, JOURNAL OF MEMBRANE SCIENCE, 642巻, 20220215
  51. ★, Ultrahigh permeation of CO2 capture using composite organosilica membranes, SEPARATION AND PURIFICATION TECHNOLOGY, 282巻, 20220201
  52. Atmospheric-pressure PECVD synthesis of polymer-supported molecular sieving silica membranes for gas separation: Effect of pore size of polymeric support, MATERIALS LETTERS, 308巻, 20220201
  53. Enhanced production of butyl acetate via methanol-extracting transesterification membrane reactors using organosilica membrane: Experiment and modeling, CHEMICAL ENGINEERING JOURNAL, 429巻, 20220201
  54. Controlled organosilica networks via metal doping for improved dehydration membranes with layered hybrid structures, SEPARATION AND PURIFICATION TECHNOLOGY, 278巻, 20220101
  55. Facile low-temperature route toward the development of polymer-supported silica-based membranes for gas separation via atmospheric-pressure plasma-enhanced chemical vapor deposition, JOURNAL OF MEMBRANE SCIENCE, 638巻, 20211115
  56. Steam recovery via nanoporous and subnanoporous organosilica membranes: The effects of pore structure and operating conditions, SEPARATION AND PURIFICATION TECHNOLOGY, 275巻, 20211115
  57. Effect of the Ti/Zr ratio on the hydrothermal and chemical stability of TiO2-ZrO2 nanofiltration membranes, SEPARATION AND PURIFICATION TECHNOLOGY, 274巻, 20211101
  58. Preparation of polysilsesquioxane reverse osmosis membranes for water desalination from tris[(ethoxysilyl)alkyl]amines by sol-gel process and interfacial polymerization, APPLIED ORGANOMETALLIC CHEMISTRY, 35巻, 11号, 202111
  59. ★, Hydrothermal stability of fluorine-induced microporous silica membranes: Effect of steam treatment conditions, AICHE JOURNAL, 67巻, 9号, 20210901
  60. Pervaporation via silicon-based membranes: Correlation and prediction of performance in pervaporation and gas permeation, AICHE JOURNAL, 67巻, 7号, 202107
  61. ★, Pore Structure Controllability and CO2 Permeation Properties of Silica-Derived Membranes with a Dual-Network Structure, INDUSTRIAL & ENGINEERING CHEMISTRY RESEARCH, 60巻, 23号, pp. 8527-8537, 20210616
  62. ★, Facile development of microstructure-engineered, ligand-chelated SiO2-ZrO2 composite membranes for molecular separations, MOLECULAR SYSTEMS DESIGN & ENGINEERING, 6巻, 6号, pp. 429-444, 20210601
  63. Microporous Nickel-Coordinated Aminosilica Membranes for Improved Pervaporation Performance of Methanol/Toluene Separation, ACS APPLIED MATERIALS & INTERFACES, 13巻, 19号, pp. 23247-23259, 20210519
  64. ★, Recent Progress in a Membrane-Based Technique for Propylene/Propane Separation, MEMBRANES, 11巻, 5号, 202105
  65. ★, Design of a SiOC network structure with oxidation stability and application to hydrogen separation membranes at high temperatures, JOURNAL OF MEMBRANE SCIENCE, 625巻, 20210501
  66. Metal-induced microporous aminosilica creates a highly permeable gas-separation membrane, MATERIALS CHEMISTRY FRONTIERS, 5巻, 7号, 20210407
  67. Multiple Amine-Contained POSS-Functionalized Organosilica Membranes for Gas Separation, MEMBRANES, 11巻, 3号, 202103
  68. Improved performance of organosilica membranes for steam recovery at moderate-to-high temperatures via the use of a hydrothermally stable intermediate layer, JOURNAL OF MEMBRANE SCIENCE, 620巻, 20210215
  69. ★, Hydrocarbon permeation properties through microporous fluorine-doped organosilica membranes with controlled pore sizes, JOURNAL OF MEMBRANE SCIENCE, 619巻, 20210201
  70. TiO2 Coatings Via Atmospheric-Pressure Plasma-Enhanced Chemical Vapor Deposition for Enhancing the UV-Resistant Properties of Transparent Plastics, ACS OMEGA, 6巻, 2号, pp. 1370-1377, 20210119
  71. Ultrafast Synthesis of Silica-Based Molecular Sieve Membranes in Dielectric Barrier Discharge at Low Temperature and Atmospheric Pressure, JOURNAL OF THE AMERICAN CHEMICAL SOCIETY, 143巻, 1号, pp. 35-40, 20210113
  72. ★, A carbon-silica-zirconia ceramic membrane with CO2 flow-switching behaviour promising versatile high-temperature H-2/CO2 separation, JOURNAL OF MATERIALS CHEMISTRY A, 8巻, 44号, pp. 23563-23573, 20201128
  73. SiC mesoporous membranes for sulfuric acid decomposition at high temperatures in the iodine-sulfur process, RSC ADVANCES, 10巻, 68号, pp. 41883-41890, 20201117
  74. ★, ゾル-ゲル法によりマイクロポーラス構造を制御したシリカ系膜のプロピレン/プロパン透過特性, 膜, 45巻, pp. 275-280, 20201101
  75. Tuning the microstructure of polycarbosilane-derived SiC(O) separation membranes via thermal-oxidative cross-linking, SEPARATION AND PURIFICATION TECHNOLOGY, 248巻, 20201001
  76. ★, Amino-decorated organosilica membranes for highly permeable CO2 capture, JOURNAL OF MEMBRANE SCIENCE, 611巻, 20201001
  77. Al2O3 nanofiltration membranes fabricated from nanofiber sols: Preparation, characterization, and performance, JOURNAL OF MEMBRANE SCIENCE, 611巻, 20201001
  78. Pervaporation removal of methanol from methanol/organic azeotropes using organosilica membranes: Experimental and modeling, JOURNAL OF MEMBRANE SCIENCE, 610巻, 20200901
  79. Filtration of surfactant-stabilized oil-in-water emulsions with porous ceramic membranes: Effects of membrane pore size and surface charge on fouling behavior, JOURNAL OF MEMBRANE SCIENCE, 610巻, 20200901
  80. Experimental study and modeling of organic solvent reverse osmosis separations through organosilica membranes, AICHE JOURNAL, 66巻, 9号, 202009
  81. High-performance molecular-separation ceramic membranes derived from oxidative cross-linked polytitanocarbosilane, JOURNAL OF THE AMERICAN CERAMIC SOCIETY, 103巻, 8号, pp. 4473-4488, 202008
  82. ★, Pore size tuning of bis(triethoxysilyl)propane (BTESP)-derived membrane for gas separation: Effects of the acid molar ratio in the sol and of the calcination temperature, SEPARATION AND PURIFICATION TECHNOLOGY, 242巻, 20200701
  83. Evaluation of experimentally obtained permeance based on module simulation: How should permeance be evaluated?, AICHE JOURNAL, 66巻, 7号, 202007
  84. ★, Pore subnano-environment engineering of organosilica membranes for highly selective propylene/propane separation, JOURNAL OF MEMBRANE SCIENCE, 603巻, 20200515
  85. ★, Development of an acetylacetonate-modified silica-zirconia composite membrane applicable to gas separation, JOURNAL OF MEMBRANE SCIENCE, 599巻, 20200401
  86. ★, Fine-tuned, molecular-composite, organosilica membranes for highly efficient propylene/propane separation via suitable pore size, AICHE JOURNAL, 66巻, 4号, 202004
  87. Development of high-performance sub-nanoporous SiC-based membranes derived from polytitanocarbosilane, JOURNAL OF MEMBRANE SCIENCE, 598巻, 20200315
  88. Energy-efficient separation of organic liquids using organosilica membranes via a reverse osmosis route, JOURNAL OF MEMBRANE SCIENCE, 597巻, 20200301
  89. Chemical-free cleaning of fouled reverse osmosis (RO) membranes derived from bis(triethoxysilyl)ethane (BTESE), JOURNAL OF MEMBRANE SCIENCE, 601巻, 20200301
  90. Phase inversion/sintering-induced porous ceramic microsheet membranes for high-quality separation of oily wastewater, JOURNAL OF MEMBRANE SCIENCE, 595巻, 20200201
  91. Ceramic-Supported Polyhedral Oligomeric Silsesquioxane-Organosilica Nanocomposite Membrane for Efficient Gas Separation, INDUSTRIAL & ENGINEERING CHEMISTRY RESEARCH, 58巻, 47号, pp. 21708-21716, 20191127
  92. Selective water vapor permeation from steam/non-condensable gas mixtures via organosilica membranes at moderate-to-high temperatures, JOURNAL OF MEMBRANE SCIENCE, 589巻, 20191101
  93. Evaluating the chemical stability of metal oxides in SO3 and applications of SiO2-based membranes to O-2/SO3 separation, JOURNAL OF THE AMERICAN CERAMIC SOCIETY, 102巻, 11号, pp. 6946-6956, 201911
  94. Vapor-permeation dehydration of isopropanol using a flexible and thin organosilica membrane with high permeance, JOURNAL OF MEMBRANE SCIENCE, 588巻, 20191015
  95. Free glycerol removal from monoglyceride using TiO2-ZrO2 nanofiltration membranes, SEPARATION AND PURIFICATION TECHNOLOGY, 224巻, pp. 366-372, 20191001
  96. TiO2-ZrO2 membranes of controlled pore sizes with different Ti/Zr ratios for nanofiltration, JOURNAL OF SOL-GEL SCIENCE AND TECHNOLOGY, 92巻, 1号, pp. 12-24, 201910
  97. Molecular Dynamics Simulation Study of Solid Vibration Permeation in Microporous Amorphous Silica Network Voids, MEMBRANES, 9巻, 10号, 201910
  98. Infrared-spectroscopic porosimetry: Development and application for characterization of hundred-nanometer-thick porous thin films, THIN SOLID FILMS, 685巻, pp. 299-305, 20190901
  99. ★, Tailoring the microstructure and permeation properties of bridged organosilica membranes via control of the bond angles, JOURNAL OF MEMBRANE SCIENCE, 584巻, pp. 56-65, 20190815
  100. Molecular dynamics simulation study on the mechanisms of liquid-phase permeation in nanopores, SEPARATION AND PURIFICATION TECHNOLOGY, 220巻, pp. 259-267, 20190801
  101. Research and development on membrane IS process for hydrogen production using solar heat, INTERNATIONAL JOURNAL OF HYDROGEN ENERGY, 44巻, 35号, pp. 19141-19152, 20190719
  102. ★, Tailoring the molecular sieving properties and thermal stability of carbonized membranes containing polyhedral oligomeric silsesquioxane (POSS)-polyimide via the introduction of norbornene, JOURNAL OF MEMBRANE SCIENCE, 582巻, pp. 59-69, 20190715
  103. ★, マイクロポーラス構造制御による高透過性分子ふるい膜の開発, 膜, 44巻, pp. 121-125, 201906
  104. Hydrothermal stability and permeation properties of TiO2-ZrO2 (5/5) nanofiltration membranes at high temperatures, SEPARATION AND PURIFICATION TECHNOLOGY, 212巻, pp. 1001-1012, 20190401
  105. ★, Effects of Calcination Condition on the Network Structure of Triethoxysilane (TRIES) and How Si-H Groups Influence Hydrophobicity Under Hydrothermal Conditions, INDUSTRIAL & ENGINEERING CHEMISTRY RESEARCH, 58巻, 9号, pp. 3867-3875, 20190306
  106. Tailoring Ultramicroporosity To Maximize CO2 Transport within Pyrimidine-Bridged Organosilica Membranes, ACS APPLIED MATERIALS & INTERFACES, 11巻, 7号, pp. 7164-7173, 20190220
  107. Effect of Sintering Temperature on Sol-Gel Synthesis of Porous Polymeric Membrane Supported Layered Hybrid Organosilica Membranes and Their Vapor Permeation Property, KAGAKU KOGAKU RONBUNSHU, 45巻, 5号, pp. 177-183, 2019
  108. Pervaporation dehydration of aqueous solutions of various types of molecules via organosilica membranes: Effect of membrane pore sizes and molecular sizes, SEPARATION AND PURIFICATION TECHNOLOGY, 207巻, pp. 108-115, 20181222
  109. Diethylenedioxane-bridged microporous organosilica membrane for gas and water separation, SEPARATION AND PURIFICATION TECHNOLOGY, 207巻, pp. 370-376, 20181222
  110. Improved thermal and oxidation stability of bis( triethoxysilyl) ethane ( BTESE)- derived membranes, and their gas- permeation properties, JOURNAL OF MATERIALS CHEMISTRY A, 6巻, 46号, pp. 23378-23387, 20181214
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  249. Gas permeation and diffusion in small and intermediate pore zeolite membranes, Studies in Surface Science and Catalysis, 170巻, pp. 847-854, 20071001
  250. A comparative study on permeation and mechanical properties of random and oriented MFI-type zeolite membranes, Microporous and Mesoporous Materials, 105巻, pp. 140-148, 20070612
  251. ★, Thermal stability improvement of MFI-type zeolite membranes with doped zirconia intermediate layer, Microporous and Mesoporous Materials,, 103巻, pp. 302-308, 20070201
  252. Permeation and separation characteristics of MFI type zeolite membranes on zirconia intermediate layer by template-free secondary growth method, Proceedings of AIChE Annual Meeting, pp. 1-8, 20061112
  253. ★, Template-free synthesis of MFI-type zeolite membranes: Permeation characteristics and thermal stability improvement of membrane structure, Journal of Membrane Science, 286巻, pp. 213-222, 20060901
  254. Permeation and separation characteristics of silicalite membranes on porous alumina support by template-free secondary growth method, Proceedings of 9th International Conference on Inorganic Membranes,, pp. 591-594, 20060401
  255. ★, Hydrogen permeation characteristics and stability of Ni-doped silica membranes in steam at high temperature, JOURNAL OF MEMBRANE SCIENCE, 271巻, 1-2号, pp. 86-93, 20060301
  256. ★, Stability of H2-permeselective Ni-doped silica membranes in steam at high temperature, JOURNAL OF CHEMICAL ENGINEERING OF JAPAN, 38巻, 11号, pp. 908-912, 200511
  257. Hydrogen separation performance and stability of Ni-doped silica membranes in high temperature steam, Proceedings of ICOM 2005, pp. 787-788, 20050401
  258. ★, Nickel-doped silica membranes for separation of helium from organic gas mixtures, SEPARATION SCIENCE AND TECHNOLOGY, 40巻, 1-3号, pp. 225-238, 2005
  259. ★, Stability of Ni-doped silica membranes for H2 separation at high temperature, Transactions of Materials Research Society of Japan, 29巻, pp. 3267-3270, 20040401
  260. Gas permeation characteristics and stability of composite silica-metal oxide membranes, Material Research Society Symposium Series, 752巻, pp. 213-218, 20030401

著書等出版物

  1. 2023年07月31日, ゾル-ゲル法の最新動向, 【Ⅲ.機能編:光,電気,化学,生体関連】第1章 マイクロポーラス構造を制御したシリカ系多孔膜, シーエムシー出版, 2023年, 202307, 単行本(学術書), 分担執筆, 金指 正言, ISBN978-4-7813-1743-4, 436
  2. 2022年04月, CO2の分離・回収・貯留の最新技術, 第2章 2.2.3 分離技術 ゾル-ゲル法によるシリカ系多孔膜のCO2分離, エヌ・ティー・エス出版, 2022年04月, 単行本(学術書), 単著, Jananese, 金指 正言, 978-4-86043-771-8, 370, 99-106
  3. 2019年07月, Current Trends and Future Developments on (Bio-)Membranes: Microporous Membrane and Membrane Reactors, Chaper 5: Gas permeation properties and pore size evaluation of microporous silica membranes, Elsevier, 2019年, 201907, 単行本(学術書), 共著, English, M. Kanezashi, T. Tsuru, 978-0-12-816350-4, 408, p.101-126
  4. 2019年04月26日, 水素の製造,輸送・貯蔵技術と材料開発事例集, 第3節 シリカ系多孔膜の細孔構造制御と水素分離への応用, 技術情報協会, 2019年, 4, 単行本(学術書), 共著, 日本語, 金指 正言,都留 稔了, ISBN978-4-86104-745-9, 415, 132-139
  5. 2018年03月, 二酸化炭素・水素分離膜の開発と応用, ゾル-ゲル法によるシリカ系膜の水素透過特性, シーエムシー出版, 2018年, 3, 単行本(学術書), 共著, Japanese, 金指正言,長澤寛規,都留稔了, ISBN978-4-7813-1321-4, 291, 111-119
  6. 2017年07月31日, ゾル-ゲルテクノロジーの最新動向, 第17章 シリカ系分子ふるい膜の細孔構造制御と透過特性, シーエムシー出版, 2017年, 201707, 単行本(学術書), 共著, Japanese, 金指 正言, 都留 稔了, ISBN978-4-7813-1258-3, 416, 12
  7. 2016年10月, Carbon Dioxide Capture: Processes, Technology and Environmental Implications, Hybrid organosilica membranes for CO2 separation under wet conditions, Nova Science Publishers, Inc., 2016年, 10, 単行本(学術書), 共著, English, X. Ren, M. Kanezashi, T. Tsuru, 978-1-63485-334-7, 326, 12
  8. 2014年12月19日, エネルギー・化学プロセスにおける膜分離技術, 第3章 第2節 ゾル-ゲル法によるシリカ膜の開発と応用技術, S&T出版, 2014年, 12, 単行本(学術書), 単著, 日本語, 金指 正言, ISBN978-4-907002-42-8, 306, 10
  9. 2014年02月24日, ゾル-ゲル法の最新応用と展望, 第6章4. ガス分離用多孔質無機膜, シーエムシー出版, 2014年, 02, 単行本(学術書), 共著, 日本語, 金指 正言, 都留 稔了, ISBN978-4-7813-0931-6, 321, 10
  10. 2014年01月21日, 最近の化学工学63「ここまできた膜分離プロセス~基礎から応用~」, 第11章 ゾル-ゲル法による多孔質セラミック膜の作製, 三恵社, 2014年, 01, 単行本(学術書), 共著, 日本語, 都留 稔了, 金指 正言, ISBN978-4-86487-178-5, 212, 11
  11. 2013年06月, Encyclopedia of Membrane Science and Technology, Sol-gel-derived silica membranes, John Wiley & Sons, 2013年, 06, 単行本(学術書), 単著, 英語, Masakoto Kanezashi, 24
  12. 2012年12月, Zeolites: Synthesis, Chemistry and Applications, Normalized Knudsen-based permeance of zeolite and silica membranes for evaluation of micro-pore sizes, Nova Science Publishers, Inc., 2012年12月, 12, 単行本(学術書), 共著, English, H. R. Lee, G. Li, M. Kanezashi, T. Yoshioka, T. Tsuru, ISBN978-1-61942-890-4, 275-284
  13. 2011年08月, Sol-Gel Process: Uniformity, Polymers and Applications, Controlling silica networks using bridged alkoxides for hydrogen separation membranes, Nova Science Publishers, 2011年, 単行本(学術書), 共著, 英語, Toshinori Tsuru, H. R. Lee, Masakoto Kanezashi, 8
  14. 2011年05月, Membrane Science and Technology Series 14, Gas permeation properties of helium, hydrogen and polar molecules through microporous silica membranes at high temperatures: Correlation with silica network structure, Elsevier, 2011年, 単行本(学術書), 共著, 英語, Masakoto Kanezashi, Toshinori Tsuru, 20

招待講演、口頭・ポスター発表等

  1. Pore size controllability and improved stability of microporous silica membranes for H2 separation, M. Kanezashi, Hydrogen Power Theoretical & Engineering Solutions International Symposium (HYPOTHESES XIX), 2024年07月17日, 招待, 英語, HYPOTHESIS XIX Hiroshima 2024 executive committee, International Conference Center Hiroshima (ICCH), プレプリント
  2. Microstructure engineering of silica-based membranes and application to gas separation at extremely low temperature, M. Kanezashi, 2nd International Congress on Separation and Purification Technology (ISPT2024), 2024年07月10日, 招待, 英語, Henan, China, プレプリント
  3. Recent progress and perspective of microporous silica membranes for molecular separation, M. Kanezashi, Department seminar at Zhengzhou University, 2024年07月07日, 招待, 英語, Department of Chemical Engineering, Zhengzhou University, Zhengzhou University, プレプリント
  4. Microstructure tailoring of ligand-modified ceramic membranes for gas separation, M. Kanezashi, 13th International Congress on Membranes and Membrane Processes (ICOM2023), 2023年07月11日, 招待, 英語, The Membrane Society of Japan, プレプリント
  5. シリカ系多孔膜の細孔径制御技術と各種ガス分離プロセスへの応用, 金指 正言, 第75回中国四国産学連携化学フォーラム, 2023年06月24日, 招待, 日本語, 日本化学会中国四国支部, プレプリント
  6. マイクロポーラス構造を制御したシリカ系多孔膜によるCO2分離, 金指 正言, 日本ゾル-ゲル学会第20回セミナー「カーボンニュートラル社会実現に向けたゾル-ゲル技術の役割」, 2023年05月30日, 招待, 日本語, 日本ゾル-ゲル学会, オンライン(web meeting), プレプリント
  7. Microstructure Engineering of Silica-based Membranes for Gas Separation, M. Kanezashi, Department seminar at National Taiwan University (NTU), 2023年04月21日, 招待, 英語, Department of Chemical Engineering, National Taiwan University (NTU), National Taiwan University (NTU), Taiwan, プレプリント
  8. ゾル-ゲル法によりマイクロポーラス構造を制御したシリカ系多孔膜の水素透過特性, 金指 正言, 第3回先端膜工学研究推進機構特定テーマフォーラム「膜を用いた水素分離の最前線」, 2022年12月22日, 招待, 日本語, 一般社団法人 先端膜工学研究推進機構, オンライン, プレプリント
  9. ゾル-ゲル法によるシリカ系多孔膜の細孔構造制御とCO2透過特性, 金指 正言, 膜によるCO2分離回収技術と研究開発動向~Direct Air Capture:DACも含めて~, 2022年08月22日, 招待, 日本語, 技術情報センター, プレプリント
  10. Molecular-level Engineering of Hybrid Inorganic-Organic Membrane via Utilization of Unsaturated Precursors, M. Kanezashi, The 13th Conference of the Aseanian Membrane Society (AMS13), 2022年07月05日, 招待, 英語, Nanyang Technological University, Singapore, プレプリント
  11. シリカ系多孔膜によるCO2透過特性, 金指 正言, 二酸化炭素分離膜開発の最新動向と今後の展望, 2022年03月10日, 招待, 日本語, 日本膜学会, オンライン開催, 発表資料
  12. Microstructure engineering of ligand-modified ceramic membranes derived from network-forming precursors, M. Kanezashi, 14th Pacific Rim Conference of Ceramic Societies (PACRIM14), 2021年12月16日, 招待, 英語, The American Ceramic Society, オンライン開催, プレプリント
  13. シリカネットワークエンジニアリングによる構造安定化と気体分離膜の開発, 金指 正言, 第21回反好会講演会, 2021年09月21日, 招待, 日本語, 化学工学会反応工学部会, 発表資料
  14. Tailoring the amorphous microporous silica structure for gas separation membrane, M. Kanezashi, 2020 Dalian University of Technology-Overseas Partner Universities Series Online Exchange Conference, 2021年01月08日, 招待, 英語, Dalian University of Technology, 発表資料
  15. Development of silica-derived molecular sieving membranes via controlling microporous structure, M. Kanezashi, AIChE Annual Meeting, 2020年11月19日, 招待, 英語, American Institute of Chemical Engineers, Virtual Meeting (Web), プレプリント
  16. Tailoring molecular sieving property and thermal stability of organic inorganic hybrid membranes for gas separation, M. Kanezashi, 13th Pacific Rim Conference of Ceramic Societies (PACRIM13), 2019年10月30日, 招待, 英語, The Ceramic Society of Japan, Okinawa, プレプリント
  17. ゾル-ゲル法によるシリカ系分子ふるい膜の細孔構造制御と透過特性, 金指 正言, 日本ゾル–ゲル学会第17回討論会, 2019年08月06日, 招待, 日本語, プレプリント
  18. ゾル-ゲル法によるシリカ系分子ふるい膜の開発と各種ガス分離プロセスへの応用, 金指 正言, JPIJS関西地区討論会, 2019年07月25日, 招待, 日本語, プレプリント
  19. Development of highly permeable molecular sieving membranes via controlling microporous structure, Masakoto Kanezashi, 9th International Symposium on Inorganic Membranes (ISIM9), 2019年07月, 招待, 英語, 発表資料
  20. ゾル-ゲル法によりネットワーク構造を制御したシリカ系膜の炭化水素透過特性, 金指正言,長澤寛規,都留稔了, 化学工学会第83年会, 2018年03月13日, 招待, 日本語, プレプリント
  21. Pore size controllability and gas permeation properties of sol-gel derived amorphous silica membranes, Masakoto Kanezashi, International Institute for Carbon-Neutral Energy Research (I2CNER) workshop 2018, 2018年02月02日, 招待, 英語, International Institute for Carbon-Neutral Energy Research (I2CNER), Kyushu University, 発表資料
  22. 炭化水素分離のためのシリカ系膜の開発, 金指 正言, 第34回ニューメンブレンテクノロジーシンポジウム, 2017年10月17日, 招待, 日本語, 日本膜学会,一般社団法人日本能率協会, 東京, 発表資料
  23. Tailoring the subnano amorphous silica network structure for development of highly permeable gas separation membranes, M. Kanezashi, The Society of Chemical Engineers, Japan (SCEJ) 49th Autumn Meeting (Joint Session of SCEJ and KIChE), 2017年09月21日, 招待, 英語, The Society of Chemical Engineers, Japan, プレプリント
  24. ゾル-ゲル法によりアモルファス構造を制御したシリカ系膜の開発と透過特性, 金指 正言, 無機膜研究センター産業化戦略協議会 第5回セミナー, 2017年05月19日, 招待, 日本語, 発表資料
  25. 橋架けアルコキシドによるオルガノシリカ膜の細孔構造制御と炭化水素透過特性, 金指正言,米田悠里,長澤寛規,都留稔了, 化学工学会第82年会, 2017年03月, 招待, 日本語, 化学工学会
  26. ゾル-ゲル法によりネットワーク構造を制御したシリカ系気体分離膜の開発, 金指 正言, 日本セラミックス協会 第29回秋季シンポジウム, 2016年09月09日, 招待, 日本語
  27. Tailoring the silica network structure for highly permeable gas separation membranes and evaluation of gas permeation properties, Masakoto Kanezashi, 7th International Symposium on Inorganic Membranes (ISIM7), 2016年07月30日, 招待, 英語
  28. シリカ系気体分離膜のネットワーク構造制御と透過特性評価, 金指 正言, 日本膜学会第38年会, 2016年05月11日, 招待, 日本語, 日本膜学会, 早稲田大学
  29. Normalized Knudsen-based Permeance (NKP)によるアモルファスシリカ膜の細孔径評価, 金指 正言, 分離工学セミナー「サブナノポア測定技術の最新動向:多孔質吸着材および分離膜の開発に向けて」, 2015年04月, 招待, 日本語, 日本膜学会,化学工学会膜分科会,化学工学会中国四国支部
  30. シリカネットワーク構造制御による新規水素分離膜の創製, 金指 正言, 化学工学会第43回秋季大会, 2011年09月, 招待, 日本語, 化学工学会
  31. Sol-gel derived Pd-SiO2 composite membranes for hydrogen separation, 金指 正言, 第20回日本MRS学術シンポジウム, 2010年12月, 招待, 日本語
  32. Sol-gel derived silica membranes for hydrogen separation, Masakoto Kanezashi, 2nd International Symposium on Inorganic Membranes, 2009年07月, 招待, 英語

受賞

  1. 2021年11月06日, 第20回(令和3年度)広島大学学長表彰 Phoenix Outstanding Researcher Award, 広島大学
  2. 2020年11月07日, 第19回(令和2年度)広島大学学長表彰 Phoenix Outstanding Researcher Award, 広島大学
  3. 2019年11月02日, 第18回(令和元年度)広島大学学長表彰 Phoenix Outstanding Researcher Award, 広島大学
  4. 2018年, Outstanding Paper Award of 2018 Journal of Chemical Engineering of Japan, Hiroshima University, Atmospheric-pressure plasma-enhanced chemical vapor deposition of hybrid silica membranes
  5. 2016年05月11日, 日本膜学会膜学研究奨励賞, 日本膜学会, シリカ系気体分離膜のネットワーク構造制御と透過特性評価
  6. 2013年, Outstanding Paper Award of 2013 Journal of Chemical Engineering of Japan, Hiroshima University, Micropore filling phase permeation of a condensable vapor in silica membranes: A molecular dynamics study
  7. 2011年03月01日, 化学工学会研究奨励賞 實吉雅郎記念賞, 化学工学会, シリカネットワーク構造制御による新規水素分離膜の創製
  8. 2005年08月, Best poster award, ICOM 2005 (International Congress on Membranes and Membrane Processes), Hydrogen separation performance and stability of Ni-doped silica membranes in high temperature steam

取得

  1. 特許権, 6935645, 2021年08月30日, ガス分離膜、ガス分離モジュール及びガス分離装置
  2. 特許権, 6842686, 2021年02月25日, 物質量測定方法、細孔径分布導出方法、物質量測定装置及び細孔径分布導出装置
  3. 特許権, 6771169, 2020年10月01日, 水蒸気を含有する混合ガス用気体分離フィルタ及びその製造方法
  4. 特許権, 6683365, 2020年03月30日, 気体分離フィルタの製造方法
  5. 特許権, 6645773, 2020年01月14日, 細孔径評価装置および細孔径評価方法
  6. 特許権, 6548215, 2019年07月15日, 分離膜及びその製造方法
  7. 特許権, 6474583, 2019年02月08日, 分離フィルタの製造方法
  8. 特許権, 6154692, 2017年06月09日, 流体分離材料及びその製造方法
  9. 特許権, 6118205, 2017年03月31日, 流体分離材料および流体分離モジュール
  10. 特許権, 5929732, 2016年05月13日, ガス分離膜及びその製造方法
  11. 特許権, 5900959, 2016年03月18日, 逆浸透膜フィルタ
  12. 特許権, 5405087, 2013年11月08日, 水素分離体及び水素分離体の製造方法
  13. 特許権, 4599557, 2010年10月08日, 気体分離膜及びその製造方法

外部資金

競争的資金等の採択状況

  1. 科学研究費助成事業(挑戦的研究(萌芽)), 超撥水性オルガノシリカ構造設計と薄膜化によるアルコール高選択透過膜の創製, 2020年, 2022年
  2. 科学研究費助成事業(挑戦的研究(萌芽)), 超耐熱性オルガノシリカ構造設計とアルカン脱水素化の革新的膜型反応システムへの応用, 2018年, 2019年
  3. 科学研究費助成事業(基盤研究(B)), アニオンドープによりサブナノ空間を精密制御した新規シリカ系分子ふるい膜の創製, 2018年, 2020年
  4. 科学研究費助成事業(基盤研究(C)), ヒドロシリル化による超耐熱性を有するSiOCネットワーク設計と気体分離膜への応用, 2015年, 2017年
  5. 科学研究費助成事業(基盤研究(C)), シリカネットワーク構造制御による超高透過性を有する二酸化炭素分離膜の創製, 2012年, 2014年
  6. 科学研究費助成事業(若手研究(B)), ゾルゲル法による超薄膜パラジウム分散型シリカ系高水素選択透過膜の開発, 2010年, 2011年
  7. 科学研究費助成事業(若手研究(B)), 新規アルコキシドを用いた超高透過性を有する水素分離膜の開発, 2008年, 2009年

社会活動

委員会等委員歴

  1. 分離技術会運営委員, 2024年07月01日, 2026年06月30日, 分離技術会
  2. 膜工学ニュース論文紹介サービス編集委員, 2020年04月01日, 9999年99月, 化学工学会 分離プロセス部会 膜工学分科会
  3. 日本ゾル-ゲル学会理事, 2020年04月01日, 9999年99月, 日本ゾル-ゲル学会
  4. 膜誌編集委員, 2019年04月01日, 9999年, 日本膜学会
  5. 化学工学誌トピックス委員, 2019年01月01日, 公益社団法人 化学工学会
  6. 中国地区化学工学懇話会幹事, 2018年04月20日, 2020年04月, 中国地区化学工学懇話会
  7. 膜工学分科会幹事(中国・四国・九州地区), 2017年04月01日, 9999年, 化学工学会膜工学分科会

学術会議等の主催

  1. 日本セラミックス協会 第29回秋季シンポジウム, 秋季シンポジウム現地実行委員, 2016年04月, 2016年09月
  2. The 7th International Symposium on Inorganic Membranes (ISIM7), 組織委員, 2016年01月, 2016年07月
  3. The 10th Conference of Aseanian Membrane Society (AMS10), 実行委員, 2015年10月, 2016年07月
  4. 日本ゾル-ゲル学会第11回討論会, 運営委員, 2013年08月
  5. ZMPC 2012 (International Symposium on Zeolites and Microporous Crystals), 運営委員, 2012年07月
  6. 日本膜学会第34年会, 組織委員, 2012年05月
  7. 膜シンポジウム2009, 運営委員, 2009年11月
  8. 化学工学会第41回秋季大会, 実行委員, 2009年09月
  9. AMS5 (The Fifth Conference of Aseanian Membrane Society), Secretariat of AMS5 special issue, 2009年07月

その他社会貢献活動(広大・部局主催含)

  1. 日本ゾル-ゲル学会第11回討論会,2013/8/1-2,広島大学,運営委員, セミナー・ワークショップ